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The Bibliography Collection is made up of bibliographies and catalogues, with Spanish and foreign assets. Begun in the second half of the 19th century, it grew considerably in the 20th century thanks to the Copyright Library Act and to the acquisition of foreign reference works.

The collection is complemented by general reference works (dictionaries, encyclopaedia, etc.) located in the Reading Room, and by the specialised bibliographies and reference works found in the Manuscripts, Fine Arts and Music rooms.